Main Cast
Jack Angel
Papa Smurf (voice)
Fred Armisen
Brainy (voice)
Hank Azaria
Gargamel (voice)
Gary Basaraba
Hefty (voice)
George López
Grouchy (voice)
Melissa Sturm
Smurfette (voice)
Anton Yelchin
Clumsy (voice)
Frank Welker
Azrael (voice)
Kirk Baily
Additional Voices (voice)
Jess Harnell
Additional Voices (voice)
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